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E. A. ZASAVITSKY, V. G. KANTSER, D. F.
MEGLEI
Charge State of Thallium Impurity and Thermoelectric Power of Semiconductor
Microwires of PbTe<Tl>
Abstract.
Results of the measurements of thermoelectric properties of thin semiconductor
microwires of Pb1-xTlxTe (x = 0.001 ¸ 0.02, d = 5 ¸ 100 mm) in the temperature
region 4.2 ¸300 K, which were obtained from solution melt by the filling of
quartz capillary with the following crystallization of material are presented.
For the samples corresponding to chemical composition with concentration of
thallium 0.0025 < x < 0.005 double change of the sign of thermoelectric power is
observed. In pure samples and samples with thal-lium concentration more than 1
at.% thermoelectric power it is positive in the whole temperature range. Various
mechanisms which can lead to observable anomalies, including Kondo-like behavior
of a non-magnetic degenerate two-level system are discussed. Obtained
experimental results let suppose that the observed anomalies can be interpreted
on the basis of model of an impurity with mixed valences. |